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TalkTalk Mobile Service Number is 0345 172 0044 available Monday – Friday, 8 am – 8 pm, Saturday- Sunday, 9 am – 6 pm. This is the TalkTalk phone number 0345 172 0044 to dial If you have any complaints about TalkTalk mobile. This is also the TalkTalk mobile service phone number 0345 172 0044 to call if you want to make a payment from your TalkTalk account.